A photon-photon quantum gate based on a single atom in an optical resonator

Two photons in free space pass each other undisturbed. This is ideal for the faithful transmission of information, but prohibits an interaction between the photons as required for a plethora of applications in optical quantum information processing. The long-standing challenge here is to realise a deterministic photon-photon gate. This requires an interaction so strong that the two photons can shift each others phase by pi. For polarisation qubits, this amounts to the conditional flipping of one photon's polarisation to an orthogonal state. So far, only probabilistic gates based on linear optics and photon detectors could be realised, as "no known or foreseen material has an optical nonlinearity strong enough to implement this conditional phase shift..." [Science 318, 1567]. Meanwhile, tremendous progress in the development of quantum-nonlinear systems has opened up new possibilities for single-photon experiments. Platforms range from Rydberg blockade in atomic ensembles to single-atom cavity quantum electrodynamics. Applications like single-photon switches and transistors, two-photon gateways, nondestructive photon detectors, photon routers and nonlinear phase shifters have been demonstrated, but none of them with the ultimate information carriers, optical qubits. Here we employ the strong light-matter coupling provided by a single atom in a high-finesse optical resonator to realise the Duan-Kimble protocol of a universal controlled phase flip (CPF, pi phase shift) photon-photon quantum gate. We achieve an average gate fidelity of F=(76.2+/-3.6)% and specifically demonstrate the capability of conditional polarisation flipping as well as entanglement generation between independent input photons. Our gate could readily perform most of the hitherto existing two-photon operations. It also discloses avenues towards new quantum information processing applications where photons are essential.Comment: 7 pages, 5 figure

Nondestructive Detection of an Optical Photon

All optical detectors to date annihilate photons upon detection, thus excluding repeated measurements. Here, we demonstrate a robust photon detection scheme which does not rely on absorption. Instead, an incoming photon is reflected off an optical resonator containing a single atom prepared in a superposition of two states. The reflection toggles the superposition phase which is then measured to trace the photon. Characterizing the device with faint laser pulses, a single-photon detection efficiency of 74% and a survival probability of 66% is achieved. The efficiency can be further increased by observing the photon repeatedly. The large single-photon nonlinearity of the experiment should enable the development of photonic quantum gates and the preparation of novel quantum states of light.Comment: published online in Science Express, 14 November 201

Photon-Mediated Quantum Gate between Two Trapped Neutral Atoms in an Optical Cavity

Quantum logic gates are fundamental building blocks of quantum computers. Their integration into quantum networks requires strong qubit coupling to network channels, as can be realized with neutral atoms and optical photons in cavity quantum electrodynamics. Here we demonstrate that the long-range interaction mediated by a flying photon performs a gate between two stationary atoms inside an optical cavity from which the photon is reflected. This single step executes the gate in $2\,\mathrm{\mu s}$. We show an entangling operation between the two atoms by generating a Bell state with 76(2)% fidelity. The gate also operates as a CNOT. We demonstrate 74.1(1.6)% overlap between the observed and the ideal gate output, limited by the state preparation fidelity of 80.2(0.8)%. As the atoms are efficiently connected to a photonic channel, our gate paves the way towards quantum networking with multiqubit nodes and the distribution of entanglement in repeater-based long-distance quantum networks.Comment: 10 pages including appendix, 5 figure

Breakdown of atomic hyperfine coupling in a deep optical-dipole trap

We experimentally study the breakdown of hyperfine coupling for an atom in a deep optical-dipole trap. One-color laser spectroscopy is performed at the resonance lines of a single $^{87}$Rb atom for a trap wavelength of 1064 nm. Evidence of hyperfine breakdown comes from three observations, namely a nonlinear dependence of the transition frequencies on the trap intensity, a splitting of lines which are degenerate for small intensities, and the ability to drive transitions which would be forbidden by selection rules in the absence of hyperfine breakdown. From the data, we infer the hyperfine interval of the $5P_{1/2}$ state and the scalar and tensor polarizabilities for the $5P_{3/2}$ state

Cavity Carving of Atomic Bell States

We demonstrate entanglement generation of two neutral atoms trapped inside an optical cavity. Entanglement is created from initially separable two-atom states through carving with weak photon pulses reflected from the cavity. A polarization rotation of the photons heralds the entanglement. We show the successful implementation of two different protocols and the generation of all four Bell states with a maximum fidelity of (90+-2)%. The protocol works for any distance between cavity-coupled atoms, and no individual addressing is required. Our result constitutes an important step towards applications in quantum networks, e.g. for entanglement swapping in a quantum repeater.Comment: 9 pages, 7 figures including Supplemen

Increased Dimensionality of Raman Cooling in a Slightly Nonorthogonal Optical Lattice

We experimentally study the effect of a slight nonorthogonality in a two-dimensional optical lattice onto resolved-sideband Raman cooling. We find that when the trap frequencies of the two lattice directions are equal, the trap frequencies of the combined potential exhibit an avoided crossing and the corresponding eigenmodes are rotated by 45 degrees relative to the lattice beams. Hence, tuning the trap frequencies makes it possible to rotate the eigenmodes such that both eigenmodes have a large projection onto any desired direction in the lattice plane, in particular, onto the direction along which Raman cooling works. Using this, we achieve two-dimensional Raman ground-state cooling in a geometry where this would be impossible, if the eigenmodes were not rotated. Our experiment is performed with a single atom inside an optical resonator but this is inessential and the scheme is expected to work equally well in other situations

Correlations and Counting Statistics of an Atom Laser

We demonstrate time-resolved counting of single atoms extracted from a weakly interacting Bose-Einstein condensate of $^{87}$Rb atoms. The atoms are detected with a high-finesse optical cavity and single atom transits are identified. An atom laser beam is formed by continuously output coupling atoms from the Bose-Einstein condensate. We investigate the full counting statistics of this beam and measure its second order correlation function $g^{(2)}(\tau)$ in a Hanbury Brown and Twiss type experiment. For the monoenergetic atom laser we observe a constant correlation function $g^{(2)}(\tau)=1.00\pm0.01$ and an atom number distribution close to a Poissonian statistics. A pseudo-thermal atomic beam shows a bunching behavior and a Bose distributed counting statistics

Heralded Storage of a Photonic Quantum Bit in a Single Atom

Combining techniques of cavity quantum electrodynamics, quantum measurement, and quantum feedback, we have realized the heralded transfer of a polarization qubit from a photon onto a single atom with 39% efficiency and 86% fidelity. The reverse process, namely, qubit transfer from the atom onto a given photon, is demonstrated with 88% fidelity and an estimated efficiency of up to 69%. In contrast to previous work based on two-photon interference, our scheme is robust against photon arrival-time jitter and achieves much higher efficiencies. Thus, it constitutes a key step toward the implementation of a long-distance quantum network.Comment: 6 pages, 4 figure

Deterministic creation of entangled atom-light Schr\"odinger-cat states

Quantum physics allows for entanglement between microscopic and macroscopic objects, described by discrete and continuous variables, respectively. As in Schr\"odinger's famous cat gedanken experiment, a box enclosing the objects can keep the entanglement alive. For applications in quantum information processing, however, it is essential to access the objects and manipulate them with suitable quantum tools. Here we reach this goal and deterministically generate entangled light-matter states by reflecting a coherent light pulse with up to four photons on average from an optical cavity containing one atom. The quantum light propagates freely and reaches a remote receiver for quantum state tomography. We produce a plethora of quantum states and observe negative-valued Wigner functions, a characteristic sign of non-classicality. As a first application, we demonstrate a quantum-logic gate between an atom and a light pulse, with the photonic qubit encoded in the phase of the light field.Comment: includes Methods and Supplementary Informatio